#+OPTIONS: auto-id:t * [[file:../README.org][Up]] :PROPERTIES: :CUSTOM_ID: h-626FBDAB-68CA-4981-9C1F-2E10BEDCD14A :END: * Introduction :PROPERTIES: :CUSTOM_ID: h-307B86F4-24F4-4387-9AE8-FE8D8E2FDAFA :END: * KKR introduction :PROPERTIES: :CUSTOM_ID: h-9E5F59BA-9F97-45B5-BEB8-F52226157FAC :END: - master-thesis speaking notes for this slide - [[file:~/src/iffgit.fz-juelich.de/phd-project-wasmer/publishing/master-thesis/notes/speaking/MScThesis_Presentation_Speaking_Notes.org::#h-cb86fd2d-4acd-4934-a5dc-d54797fbc4b6][4 KKR-GF]] - KKR SCF cycle - [[file:~/Desktop/Studium/Kurse_RWTH/DensityFunctionalTheory/20W/Lecture 17-20 Electronic Struct___eudopotential, PAW, FLAPW, KKR/Lecture20_KKRGF-Method.pdf][dft20 lecture 20 KKR]] - p. 18 - 1) potential V -> solutions R, H - from [[https://iffmd.fz-juelich.de/jAngJ9qIQgSwPObGOSU1dw#][iffMD KKRimp tutorial]]: this is the single-site problem - from dft20 p.27: secular equation: local solution of TISE in each cell with basis RL YL - from [[https://iffmd.fz-juelich.de/jAngJ9qIQgSwPObGOSU1dw#][iffMD KKRimp tutorial]]: t = V + V G0 t = \int_V \sum_L J V R - 2) Algebraic Dyson equation -> structural GF - the ADE IS the SGF - the SGF contains all possible scattering paths btw any two cells - Sol found by Fourier transform (k-space), matrix inv, back-transform (otherwise infinite sum) - from msc2a. for KKRimp, one gets the impurity region block GII from impurity SGF inversion in real space and discarding all blocks GRI, GIR, GRR. Host G0 enters as a boundary condition but does not change. - 3) GF = SiSca + Musca(structural GF) - From lit-rev - kkr.org - [[file:~/src/iffgit.fz-juelich.de/phd-project-wasmer/learn/literature-review/notes/topics/kkr.org::#h-5A792112-F416-4096-8067-E61A5BC02A38][blugelDensityFunctionalTheory2006 - 6 The Green function method of Korringa, Kohn and Rostoker]] #+begin_quote In order to solve the Schrödinger equation, the scattering properties of each scattering center (atom) are determined in a first step and described by a scattering matrix, while the multiple-scattering by all atoms in the lattice is determined in a second step by demanding that the incident wave at each center is the sum of the outgoing waves from all other centers. In this way, a separation between the potential and geometric properties is achieved. A further significant development of the KKR scheme came when it was reformulated as a KKR Green function method [75, 76]. By separating the single-site scattering problem from the multiple-scattering effects, the method is able to produce the crystal Green function efficiently by relating it to the Green function of free space via the Dyson equation. In a second step the crystal Green function can be used as a reference in order to calculate the Green function of an impurity in the crystal [77], again via a Dyson equation. This way of solving the impurity problem is extremely efficient, avoiding the construction of huge supercells which are needed in wavefunction methods. #+end_quote - Observables and electron density - from lit-rev - kkr.org #+begin_quote [...] charge density \(n(\bm{r})\) can be directly expressed by an energy integral over the imaginary part of the Green function #+end_quote - from msc2a_theory #+begin_quote The integral sums over all occupied states up to the Fermi energy \(E_F\) at zero absolute temperature #+end_quote - expensive energy integrals are calculated efficiently via contour integration (less E points) - Some KKR applications besides impurity embeddings - surfaces, layered systems, transport and spectroscopic properties, linear-scaling DFT with accurate long-range interactions (KKRnano), disordered systems (CPA), conventional superconductivity (BdG-DFT), etc.